Hi @Angel487 ,
Thank you for your interest in the NXP MIMXRT product, I would like to provide service for you.
I checked the LPSPI IP module, from the register, just can select one PCS pin:

TCR register:

If you want more than one pin as the SPI_CS function.
Just the LPSPI IP hardware, no register to select it.
So, maybe still need to use the GPIO method.
You mentioned:
I also tried to drive the pins as normal GPIOs, but this results in an out of timing behavior of CS.
What's the detail situation? Which timing behavior is out?
Can you share some wave about it?
If you think the normal GPIO speed is slow, you can use the fast GPIO:
https://www.cnblogs.com/henjay724/p/15518705.html
If just the CS area is not correct, it is related to your GPIO CS code insert area, you need to go to the fsl_lpspi to add it.
With it helps you!
Best Regards,
Kerry