Hello Jonathan ,
OUT0~OUT7 all can be used as GPIO function. But these pins are multiplexed. You should do 2 steps for GPIO:
1. Enable them on corresponding bit in Register "PinEn"


[note]
You can try to write 1 at bit0, and check if GPO function is enabled, otherwise write 0, please! I also didn't find detailed description on 1 or 0 for GPO function.
2. Output High Or Low in Register "8.15.2 PinOut"


Write 1 on related bit, High level should be output, otherwise Low level.
In addtion, if your LED needs 1-3mA, it is no problem to driver them diretly via GPO. if higher current is needed, you can add a MOSFET to driver LEDs.
Have a nice day!
Best Regards,
Weidong Sun