HI,
Based on LPC5528-EVK board, you want to use the FLEXCOMM7 as SPI module.

This is the pin assignment:
PIO1_2 FC7_SCK
PIO1_3 FC7_MISO
PIO0_26 FC7_MOSI
PIO1_1 FC7_SSEL1
In the pin_mux.c in SDK project, I suppose you can add the api function so that you can configure the pin as FC7 SPI pin.
For the PIO1_1, when the func is 5, the pin will function as HS_SPI_SSEL1

So you can use the code to assign the FUNC as 5
#define IOCON_PIO_FUNC5 5
CLOCK_EnableClock(kCLOCK_Iocon);
const uint32_t port1_pin1_config = (/* Pin is configured as HS_SPI_SSEL1 */
IOCON_PIO_FUNC5 |
/* No addition pin function */
IOCON_PIO_MODE_INACT |
/* Standard mode, output slew rate control is enabled */
IOCON_PIO_SLEW_STANDARD |
/* Input function is not inverted */
IOCON_PIO_INV_DI |
/* Enables digital function */
IOCON_PIO_DIGITAL_EN |
/* Open drain is disabled */
IOCON_PIO_OPENDRAIN_DI);
IOCON_PinMuxSet(IOCON, 1U, 1U, port1_pin1_config);
Pls follow up the above line to configure the other pins such as PIO1_2, PIO1_3 and PIO0_26
BTW, you can not use GPIO_PinWrite()/GPIO_PinRead(), they are used to write or read a pin logic only when you have configure the pin as GPIO function.
Hope it can help you
BR
XiangJun Rong