Hello ChrisN,
You can refer to the XIP demos under SDK, for example hello_world_qspi_xip.
Add spifi programming algorithm in Flash Download:
Alice_Yang_0-1633746268334.png
If use J-link debugger, configure as below:
Alice_Yang_1-1633746345872.png
About the two SPIFI flash, you can check their datasheet, and try to use. If there is no problem when using MCUXpresso IDE, It also should be work with KEIL.
BR
Alice