Hi Chris Westervelt,
To set the security you will have to modify the address 0x0_040C this address is a byte long.

I think the important thing here for you is the
- KEYEN.- this is the Key enable, you can set a backdoor key to acces . this key will temporary unsecure the MCU so you can modifiy whatever you need and when you reset the MCU will be secured.
- SEC.- When this is Enabled the MCU is going to be secured
Please check the http://www.nxp.com/assets/documents/data/en/reference-manuals/K82P121M150SF5RM.pdf reference manual in the chapter 10.
Please let me know if you have more questions.
(Please try to set the mass erase to enable otherwise, if for some reason you forgot your backdoor key you can erase the MCU and use it again)
Have a great day
Best Regards
Jonathan