Hi, Christie,
Of course, you can use FlexBus to extend NOR flash and normal SRAM, as you said the connection needs more pins, it needs address bus, data bus and control bus.
The K66F and KV58F has spi module, but it is normal spi module instead of qspi or hyperbus, in other words, KV58 and K66 can not connect with qspi or hyperbus SRAM or flash.
We have Kinetis K8x, they have on-chip qspi module, which can connect with flash or SRAM with qspi interface.
Hope it can help you
BR
Xiangjun rong