From reading the data sheet, it looks like the slave device will send out the most significant bits of the pressure data first, for clock polarity: the clock starts at a low state and becomes active on high, for clock phase: data is read on the clock's first edge, clock frequency should be set in between 50-800 KHz; I have it at 500 KHz. I set all of these in the SPI_MasterGetDefaultConfig function.
Attached to this response are images of readings from the oscilloscope. Something odd is that with the high-speed SPI that I'm trying to use, the chip select signal (in purple) never gets pulled down, also the clock signal (in yellow) only oscillates up to ~1.5V, and the MISO signal (in blue) just alternates between 1 and 0.
I ran an example using the "normal" SPI using FLEXCOMM3, and it was able to work just fine. If you look at the attached image, you can see the chip select signal getting pulled down, the clock oscillating from 0V to 3V, and the MISO signal producing reasonable signals besides just alternating between 1 and 0.
I do not know why the high-speed SPI signal is behaving in such an odd way.