Hi,
I did a test based on MCUXpresso SDK interrupt_b2b_master demo.
I make below change with the code:
uint32_t masterRxData[TRANSFER_SIZE] = {0U};
/*Master config*/
masterConfig.baudRate = TRANSFER_BAUDRATE;
masterConfig.bitsPerFrame = 40; //8;
masterConfig.cpol = kLPSPI_ClockPolarityActiveHigh;
masterConfig.cpha = kLPSPI_ClockPhaseFirstEdge;
masterConfig.direction = kLPSPI_MsbFirst;
masterTxData[0] = 0x11223344;
masterTxData[1] = 0x55;
I could get below transfer siganl from captured scope:

So, the LPSPI module is set to MSB first it will send your expecet data.
Have a great day,
Mike
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