The eLBC clock is derived from the platform clock (can be 1/8, 1/16, 1/32). So because you already has maximum of the platform clock frequency you cannot increase eLBC clok by sysclock frequency increasing.
The LCRR register (LCRR[CLKDIV]) controls eLBC clock:
“CLKDIV Clock divider. Sets the frequency ratio between the platform clock and the local bus clock. Only the values shown below are allowed. Note that the reset value of CLKDIV depends on the RCW source configuration(cfg_rcw_src[0:4]).
00000-00001 Reserved
00010 8
00011 Reserved
00100 16
00101-00111 Reserved
01000 32
01001-11111 Reserved
NOTE: It is critical that no transactions are being executed via the local bus while CLKDIV is being modified. As such, prior to modification, the user must ensure that code is not executing out of the
local bus. Once LCRR[CLKDIV] is written, the register should be read, and then an isync should be executed.”
Take into account that the specifications limit eLBC clock to 100 MHz.